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Atomic and Molecular Optics
Contents
Atomic and Molecular Optics
|
16 Article(s)
Reconstructing coherent dynamics of bound states induced by strong attosecond XUV pulses
Lijuan Jia, Mingqing Liu, Xinqiang Wang, Long Xu, Peiguang Yan, Wei-Chao Jiang, and Libin Fu
We propose a scheme that utilizes weak-field-induced quantum beats to investigate the electronic coherences of atoms driven by a strong attosecond extreme ultraviolet (XUV) pulse. The technique involves using a strong XUV pump pulse to excite and ionize atoms and a time-delayed weak short pulse to probe the photoelectron signal. Our theoretical analysis demonstrates that the information regarding the bound states, initiated by the strong pump pulse, can be precisely reconstructed from the weak-field-induced quantum beat spectrum. To examine this scheme, we apply it to the attosecond XUV laser-induced ionization of hydrogen atoms by solving a three-dimensional time-dependent Schrödinger equation. This work provides an essential reference for reconstructing the ultrafast dynamics of bound states induced by strong XUV attosecond pulses.
We propose a scheme that utilizes weak-field-induced quantum beats to investigate the electronic coherences of atoms driven by a strong attosecond extreme ultraviolet (XUV) pulse. The technique involves using a strong XUV pump pulse to excite and ionize atoms and a time-delayed weak short pulse to probe the photoelectron signal. Our theoretical analysis demonstrates that the information regarding the bound states, initiated by the strong pump pulse, can be precisely reconstructed from the weak-field-induced quantum beat spectrum. To examine this scheme, we apply it to the attosecond XUV laser-induced ionization of hydrogen atoms by solving a three-dimensional time-dependent Schrödinger equation. This work provides an essential reference for reconstructing the ultrafast dynamics of bound states induced by strong XUV attosecond pulses.
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Chinese Optics Letters
Publication Date: Feb. 21, 2024
Vol. 22, Issue 2, 020201 (2024)
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Momentum filtering scheme of cooling atomic clouds for the Chinese Space Station
Hui Li, Biao Wu, Jiachen Yu, Xiaolong Yuan, Xiaoji Zhou, Bin Wang, Weibiao Chen, Wei Xiong, and Xuzong Chen
To obtain cold atom samples with temperatures lower than 100 pK in the cold atom physics rack experiment of the Chinese Space Station, we propose to use the momentum filtering method for deep cooling of atoms. This paper introduces the experimental results of the momentum filtering method verified by our ground testing system. In the experiment, we designed a specific experimental sequence of standing-wave light pulses to control the temperature, atomic number, and size of the atomic cloud. The results show that the momentum filter can effectively and conveniently reduce the temperature of the atomic cloud and the energy of Bose–Einstein condensation, and can be flexibly combined with other cooling methods to enhance the cooling effect. This work provides a method for the atomic cooling scheme of the ultra-cold atomic system on the ground and on the space station, and shows a way of deep cooling atoms.
To obtain cold atom samples with temperatures lower than 100 pK in the cold atom physics rack experiment of the Chinese Space Station, we propose to use the momentum filtering method for deep cooling of atoms. This paper introduces the experimental results of the momentum filtering method verified by our ground testing system. In the experiment, we designed a specific experimental sequence of standing-wave light pulses to control the temperature, atomic number, and size of the atomic cloud. The results show that the momentum filter can effectively and conveniently reduce the temperature of the atomic cloud and the energy of Bose–Einstein condensation, and can be flexibly combined with other cooling methods to enhance the cooling effect. This work provides a method for the atomic cooling scheme of the ultra-cold atomic system on the ground and on the space station, and shows a way of deep cooling atoms.
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Chinese Optics Letters
Publication Date: Aug. 08, 2023
Vol. 21, Issue 8, 080201 (2023)
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Phase dependence of third-order harmonic generation in gases induced by two-color laser field
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Editors' Pick
Congsen Meng, Pan Song, Zhihui Lyu, Xiaowei Wang, Dongwen Zhang, Zengxiu Zhao, and Jianmin Yuan
We experimentally demonstrate third-harmonic generation (THG) in gases ionized by a femtosecond laser pulse superimposed on its second-harmonic (SH). The mechanism of THG has been investigated, and it demonstrates that a third-order nonlinear process dominates at low pump intensity. Asymmetric third-harmonic (TH) spectra are observed at different time delays in two color fields, which are attributed to the process of the four-wave mixing (FWM) of the broad spectrum of pump pulses. A joint measurement on the terahertz (THz) and the TH is performed. It reveals that the optimized phase for the THG jumps from 0 to 0.5π as the pump intensity increases, which is different from the THz being a constant, and indicates that the THG arises from the nonlinearity of the third-order bound electrons to the tunnel-ionization current.
We experimentally demonstrate third-harmonic generation (THG) in gases ionized by a femtosecond laser pulse superimposed on its second-harmonic (SH). The mechanism of THG has been investigated, and it demonstrates that a third-order nonlinear process dominates at low pump intensity. Asymmetric third-harmonic (TH) spectra are observed at different time delays in two color fields, which are attributed to the process of the four-wave mixing (FWM) of the broad spectrum of pump pulses. A joint measurement on the terahertz (THz) and the TH is performed. It reveals that the optimized phase for the THG jumps from 0 to 0.5π as the pump intensity increases, which is different from the THz being a constant, and indicates that the THG arises from the nonlinearity of the third-order bound electrons to the tunnel-ionization current.
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Chinese Optics Letters
Publication Date: May. 06, 2023
Vol. 21, Issue 5, 050201 (2023)
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Rydberg electromagnetically induced transparency in
40
K ultracold Fermi gases
Guoqi Bian, Biao Shan, Lianghui Huang, and Jing Zhang
We report the measurement of the electromagnetically induced transparency (EIT) with Rydberg states in ultracold K40 Fermi gases, which is obtained through a two-photon process with the ladder scheme. Rydberg–EIT lines are obtained by measuring the atomic losses instead of the transmitted probe beam. Based on the laser frequency stabilization locking to the superstable cavity, we study the Rydberg–EIT line shapes for the 37s and 35d states. We experimentally demonstrate the significant change in the Rydberg–EIT spectrum by changing the principal quantum number of the Rydberg state (n=37/52 and l=0). Moreover, the transparency peak position shift is observed, which may be induced by the interaction of the Rydberg atoms. This work provides a platform to explore many interesting behaviors involving Rydberg states in ultracold Fermi gases.
We report the measurement of the electromagnetically induced transparency (EIT) with Rydberg states in ultracold K40 Fermi gases, which is obtained through a two-photon process with the ladder scheme. Rydberg–EIT lines are obtained by measuring the atomic losses instead of the transmitted probe beam. Based on the laser frequency stabilization locking to the superstable cavity, we study the Rydberg–EIT line shapes for the 37s and 35d states. We experimentally demonstrate the significant change in the Rydberg–EIT spectrum by changing the principal quantum number of the Rydberg state (n=37/52 and l=0). Moreover, the transparency peak position shift is observed, which may be induced by the interaction of the Rydberg atoms. This work provides a platform to explore many interesting behaviors involving Rydberg states in ultracold Fermi gases.
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Chinese Optics Letters
Publication Date: Aug. 30, 2023
Vol. 21, Issue 10, 100201 (2023)
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Automatic, long-term frequency-stabilized lasers with sub-hertz linewidth and 10
−16
frequency instability
Chengzhi Yan, Haosen Shi, Yuan Yao, Hongfu Yu, Yanyi Jiang, and Longsheng Ma
We report two ultra-stable laser systems automatically frequency-stabilized to two high-finesse optical cavities. By employing analog-digital hybrid proportional integral derivative (PID) controllers, we keep the merits of wide servo bandwidth and servo accuracy by using analog circuits for the PID controller, and, at the same time, we realize automatic laser frequency locking by introducing digital logic into the PID controller. The lasers can be automatically frequency-stabilized to their reference cavities, and it can be relocked in 0.3 s when interruption happens, i.e., blocking and unblocking the laser light. These automatic frequency-stabilized lasers are measured to have a frequency instability of 6×10-16 at 1 s averaging time and a most probable linewidth of 0.3 Hz. The laser systems were tested for continuous operation over 11 days. Such ultra-stable laser systems in long-term robust operation will be beneficial to the applications of optical atomic clocks and precision measurement based on frequency-stabilized lasers.
We report two ultra-stable laser systems automatically frequency-stabilized to two high-finesse optical cavities. By employing analog-digital hybrid proportional integral derivative (PID) controllers, we keep the merits of wide servo bandwidth and servo accuracy by using analog circuits for the PID controller, and, at the same time, we realize automatic laser frequency locking by introducing digital logic into the PID controller. The lasers can be automatically frequency-stabilized to their reference cavities, and it can be relocked in 0.3 s when interruption happens, i.e., blocking and unblocking the laser light. These automatic frequency-stabilized lasers are measured to have a frequency instability of 6×10-16 at 1 s averaging time and a most probable linewidth of 0.3 Hz. The laser systems were tested for continuous operation over 11 days. Such ultra-stable laser systems in long-term robust operation will be beneficial to the applications of optical atomic clocks and precision measurement based on frequency-stabilized lasers.
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Chinese Optics Letters
Publication Date: May. 26, 2022
Vol. 20, Issue 7, 070201 (2022)
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Dark state atoms trapping in a magic-wavelength optical lattice near the nanofiber surface
Dianqiang Su, Xiateng Qin, Yuan Jiang, Kaidi Jin, Zhonghua Ji, Yanting Zhao, Liantuan Xiao, and Suotang Jia
We report the experimental realization of dark state atoms trapping in a nanofiber optical lattice. By applying the magic-wavelength trapping potentials of cesium atoms, the AC Stark shifts are strongly suppressed. The dark magneto-optical trap efficiently transfers the cold atoms from bright (6S1/2, F = 4) into dark state (6S1/2, F = 3) for hyperfine energy levels of cesium atoms. The observed transfer efficiency is as high as 98% via saturation measurement. The trapping lifetime of dark state atoms trapped by a nanofiber optical lattice is also investigated, which is the key element for realizing optical storage. This work contributes to the manipulation of atomic electric dipole spin waves and quantum information storage for fiber networks.
We report the experimental realization of dark state atoms trapping in a nanofiber optical lattice. By applying the magic-wavelength trapping potentials of cesium atoms, the AC Stark shifts are strongly suppressed. The dark magneto-optical trap efficiently transfers the cold atoms from bright (6S1/2, F = 4) into dark state (6S1/2, F = 3) for hyperfine energy levels of cesium atoms. The observed transfer efficiency is as high as 98% via saturation measurement. The trapping lifetime of dark state atoms trapped by a nanofiber optical lattice is also investigated, which is the key element for realizing optical storage. This work contributes to the manipulation of atomic electric dipole spin waves and quantum information storage for fiber networks.
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Chinese Optics Letters
Publication Date: Nov. 19, 2021
Vol. 20, Issue 2, 020201 (2022)
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Frequency control of a lattice laser at 759 nm by referencing to Yb clock transition at 578 nm
Yaqin Hao, Yuan Yao, Haosen Shi, Hongfu Yu, Yanyi Jiang, and Longsheng Ma
We present the frequency control of a 759 nm laser as a lattice laser for an ytterbium (Yb) optical clock. The frequency stability and accuracy are transferred from the Yb optical clock via an optical frequency comb. Although the comb is frequency-stabilized on a rubidium microwave clock, the frequency instability of the 759 nm laser is evaluated at the 10-15 level at 1 s averaging time. The frequency of the 759 nm laser is controlled with an uncertainty within 1 Hz by referencing to the Yb clock transition. Such a frequency-controlled 759 nm laser is suitable for Yb optical clocks as the lattice laser. The technique of laser frequency control can be applied to other lasers in optical clocks.
We present the frequency control of a 759 nm laser as a lattice laser for an ytterbium (Yb) optical clock. The frequency stability and accuracy are transferred from the Yb optical clock via an optical frequency comb. Although the comb is frequency-stabilized on a rubidium microwave clock, the frequency instability of the 759 nm laser is evaluated at the 10-15 level at 1 s averaging time. The frequency of the 759 nm laser is controlled with an uncertainty within 1 Hz by referencing to the Yb clock transition. Such a frequency-controlled 759 nm laser is suitable for Yb optical clocks as the lattice laser. The technique of laser frequency control can be applied to other lasers in optical clocks.
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Chinese Optics Letters
Publication Date: Sep. 23, 2022
Vol. 20, Issue 12, 120201 (2022)
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Ultranarrow bandwidth Faraday atomic filter approaching natural linewidth based on cold atoms
Wei Zhuang, Yang Zhao, Shaokai Wang, Zhanjun Fang, Fang Fang, and Tianchu Li
An ultranarrow bandwidth Faraday atomic filter is realized based on cold Rb87 atoms. The atomic filter operates at 780 nm on the 52S1/2, F=2 to 52P3/2, F′=3 transition with a bandwidth of 7.1(8) MHz, which is approaching the natural linewidth of the transition. The peak transmission achieves 2.6(3)% by the multi-pass probe method. This atomic filter based on cold atoms may find potential applications in self-stabilizing lasers in the future.
An ultranarrow bandwidth Faraday atomic filter is realized based on cold Rb87 atoms. The atomic filter operates at 780 nm on the 52S1/2, F=2 to 52P3/2, F′=3 transition with a bandwidth of 7.1(8) MHz, which is approaching the natural linewidth of the transition. The peak transmission achieves 2.6(3)% by the multi-pass probe method. This atomic filter based on cold atoms may find potential applications in self-stabilizing lasers in the future.
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Chinese Optics Letters
Publication Date: Mar. 10, 2021
Vol. 19, Issue 3, 030201 (2021)
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Uncertainty evaluation of the second-order Zeeman shift of a transportable
87
Rb atomic fountain clock
Henan Cheng, Siminda Deng, Zhen Zhang, Jingfeng Xiang, Jingwei Ji, Wei Ren, Tang Li, Qiuzhi Qu, Liang Liu, and Desheng Lü
In this article, taking advantage of the special magnetic shieldings and the optimal coil design of a transportable Rb atomic fountain clock, the intensity distribution in space and the fluctuations with time of the quantization magnetic field in the Ramsey region were measured using the atomic magneton-sensitive transition method. In an approximately 310 mm long Ramsey region, a peak-to-peak magnetic field intensity of a 0.74 nT deviation in space and a 0.06 nT fluctuation with time were obtained. These results correspond to a second-order Zeeman frequency shift of approximately (2095.5±5.1)×10-17. This is an essential step in advancing the total frequency uncertainty of the fountain clock to the order of 10-17.
In this article, taking advantage of the special magnetic shieldings and the optimal coil design of a transportable Rb atomic fountain clock, the intensity distribution in space and the fluctuations with time of the quantization magnetic field in the Ramsey region were measured using the atomic magneton-sensitive transition method. In an approximately 310 mm long Ramsey region, a peak-to-peak magnetic field intensity of a 0.74 nT deviation in space and a 0.06 nT fluctuation with time were obtained. These results correspond to a second-order Zeeman frequency shift of approximately (2095.5±5.1)×10-17. This is an essential step in advancing the total frequency uncertainty of the fountain clock to the order of 10-17.
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Chinese Optics Letters
Publication Date: Dec. 10, 2021
Vol. 19, Issue 12, 120201 (2021)
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Molecular orientation induced by H
+
collision and modulated with combined fields
Zhiwei Ge, Xuequn Hou, Yu Zhao, and Qingtian Meng
We take H++CO as a prototype to analyze the effect of ion or proton collision on molecular orientation modulated by a two-color shaped pulse combined with the time-delayed terahertz (THz) pulse. Through examining the effect of ion collision on the molecular orientation, we found that when the impact parameter and collisional velocity have weak inverse influences on the maximal orientation degree, the appropriate two-color and THz field intensity employed can improve the molecular orientation degree. The carrier envelope phase and frequency of the THz laser pulse as well as the temperature also have certain influence on the collision-induced molecular orientation.
We take H++CO as a prototype to analyze the effect of ion or proton collision on molecular orientation modulated by a two-color shaped pulse combined with the time-delayed terahertz (THz) pulse. Through examining the effect of ion collision on the molecular orientation, we found that when the impact parameter and collisional velocity have weak inverse influences on the maximal orientation degree, the appropriate two-color and THz field intensity employed can improve the molecular orientation degree. The carrier envelope phase and frequency of the THz laser pulse as well as the temperature also have certain influence on the collision-induced molecular orientation.
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Chinese Optics Letters
Publication Date: Nov. 10, 2021
Vol. 19, Issue 11, 110201 (2021)
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